Synfacts 2008(3): 0235-0235  
DOI: 10.1055/s-2008-1042749
Synthesis of Heterocycles
© Georg Thieme Verlag Stuttgart · New York

Synthesis of Chiral Pyridyl Alcohols by Cyclotrimerization

Contributor(s):Victor Snieckus, Wei Gan
B. Heller*, D. Redkin, A. Gutnov, C. Fischer, W. Bonrath, R. Karge, M. Hapke*
Leibniz-Institut für Katalyse e.V. an der Universität Rostock and ChiroBlock GmbH, Wolfen, Germany; DSM Nutritional Products Ltd., Basel, Switzerland
Synthesis of Chiral Pyridyl Alcohols Using a Two-Step Catalytic Approach
Synthesis  2008,  69-74  
Further Information

Publication History

Publication Date:
21 February 2008 (online)


Significance

Reported is a synthesis of chiral pyridyl alcohols by a two-step reaction. In the first step, catalyst (R,R)-A leads to the S-enantiomers while (S,S)-A results in the formation of the R-enantiomers. The enantiomeric excess of O-tri­methylsilylcyanohydrins B was retained in the final products after Co-catalyzed cyclotrimerization and desilylation.

Comment

Chiral pyridyl alcohols have seen applications as catalysts and ligands in asymmetric reactions such as the epoxidation of allylic alcohols (J. M. Hawkins, K. B. Sharpless Tetrahedron Lett. 1987, 28, 2825), the nucleophilic addition of dialkylzinc reagents to aldehydes (M. Ishizaki, O. Hoshino Tetrahedron: Asymmetry 1994, 5, 1901), and have served as key intermediates for drugs, for example (R,S)-mefloquine. The standard access to chiral pyridyl alcohols includes hydrogenation of pyridyl acetones (C.-Y. Chen et al. Org. Lett. 2003, 5, 5039) and resolution of racemic ­pyridyl alcohols (C.-Y. Mazet et al. Org. Lett. 2006, 8, 1879). The Co-catalyzed cyclo­trimerization of chiral cyanohydrin approach was reported previously (G. Chelucci et al. Tetrahedron: Asymmetry 1994, 5, 1973) with disadvantages of a three-step preparation of cyanohydrin precursors and high temperature (120 ºC) reaction conditions.